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Enhancement of the electrocatalytic oxidation of antibiotic wastewater over the conductive black carbon-PbO

Xiangyu Wang, Yu Xie, Guizhen Yang, Jiming Hao, Jun Ma, Ping Ning

Frontiers of Environmental Science & Engineering 2020, Volume 14, Issue 2, doi: 10.1007/s11783-019-1201-9

Abstract: • A novel conductive carbon black modified lead dioxide electrode is synthesized. • The modified PbO2(PbO2).It was observed that the as-prepared conductive carbon black modified electrode (C-PbO2) exhibited anenhanced electrocatalytical performance and more stable structure than a pristine PbO2 electrode, andthe removal efficiency of metronidazole (MNZ) and COD by a 1.0% C-PbO2 electrode at optimal conditions

Keywords： Conductive carbon black PbO2sub> electrode Metronidazole Electrochemical oxidation Box-Behnken

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NiCo2O4@quinone-rich N–C core–shell nanowires as composite electrode for electric double layer capacitor

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 4, Pages 373-386 doi: 10.1007/s11705-022-2223-6

Abstract: >2sub>O4sub> nanowires were firstly grown on the substrate of active carbon cloth to provideThen, the quinone-rich nitrogen-doped carbon shell structure was formed around NiCo2sub>O4sub> nanowires, and the obtained composite was used as electrode for electric double layer capacitorThe results showed that the composite electrode displayed an area-specific capacitance of 1794 mF∙cm^–2 at the current density of 1 mA∙cm^–2.

Keywords： carbon cloth NiCo2sub>O4sub> nanowires core−shell structure quinone-rich electric double

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Construction of nitrogen-doped carbon cladding LiMnO film electrode with enhanced stability for electrochemically

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 12, Pages 2050-2060 doi: 10.1007/s11705-023-2343-7

Abstract: Reducing the dissolution of Mn from LiMn2sub>O4sub> (LMO) and enhancing the stability of>2sub> gas to achieve the above purpose.LMO film electrode.electrode after 10 cycles.separation factor was 118.38 for Li⁺ toward Mg²⁺ in simulated brine.

Keywords： LiMn2sub>O4sub> lithium extraction surface coating cyclic stability Mn dissolution

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Construction of NiCoO nanoflake arrays on cellulose-derived carbon nanofibers as a freestanding electrode

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 6, Pages 691-703 doi: 10.1007/s11705-022-2268-6

Abstract: superior electrical conductivity of 31.2 S·cm^–1 and larger specific surface area of 35.61 m^2–1, specific surface area of 12 m^{2sub>2sub>O4sub> nanoflake arrays are grown uniformly on the cellulose-based carbonThe as-prepared cellulose-based carbon nanofibers/NiCo2sub>O4sub> nanoflake arrays are>2sub>O4sub> deliver a high energy density of 62 W·h·kg^–1 at a power density of 1200}

Keywords： cellulose carbon nanofibers NiCo2sub>O4sub> supercapacitors

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A 3D porous WP2 nanosheets@carbon cloth flexible electrode for efficient electrocatalytic hydrogen evolution

Mingyu Pi, Xiaodeng Wang, Dingke Zhang, Shuxia Wang, Shijian Chen

Frontiers of Chemical Science and Engineering 2018, Volume 12, Issue 3, Pages 425-432 doi: 10.1007/s11705-018-1726-7

Abstract:

Self-standing porous WP2sub> nanosheet arrays on carbon fiber cloth (WP2sub> NSs/CC)were synthesized and used as a 3D flexible hydrogen evolution electrode.Because of its 3D porous nanoarray structure, the WP2sub> NSs/CC exhibits a remarkable catalyticOur work makes the present WP2sub> NSs as a promising electrocatalyst for hydrogen evolution and

Keywords： WP2sub> nanosheet arrays hydrogen evolution electrocatalyst flexible electrode

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Dielectric barrier micro-plasma reactor with segmented outer electrode for decomposition of pure CO

Baowei Wang, Xiaoxi Wang, Bo Zhang

Frontiers of Chemical Science and Engineering 2021, Volume 15, Issue 3, Pages 687-697 doi: 10.1007/s11705-020-1974-1

Abstract: Compared with other types of dielectric barrier discharge plasma reactors, the proposed segmented outer electrodeconversion can be attributed mainly to the enhanced corona discharge caused by the fringe effect at electrode

Keywords： CO2sub> decomposition dielectric barrier discharge segmented outer electrodes electrical analysis

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Rh2sub>O3sub>/hexagonal CePO4sub> nanocatalysts for N2sub>O decomposition

Huan Liu, Zhen Ma

Frontiers of Chemical Science and Engineering 2017, Volume 11, Issue 4, Pages 586-593 doi: 10.1007/s11705-017-1659-6

Abstract: Hexagonal CePO nanorods were prepared by a precipitation method and hexagonal CePO nanowires were prepared by hydrothermal synthesis at 150 °C. Rh(NO ) was then used as a precursor for the impregnation of Rh O onto these CePO materials. The Rh O supported on the CePO nanowires was much more active for the catalytic decomposition of N O than the Rh O supported on CePO nanorods. The stability of both catalysts as a function of time on stream was studied and the influence of the co-feed (CO , O , H O or O /H O) on the N O decomposition was also investigated. The samples were characterized by N adsorption-desorption, inductively coupled plasma optical emission spectroscopy, X-ray diffraction, transmission electron microscopy, X-ray photoelectron microscopy, hydrogen temperature-programmed reduction, oxygen temperature-programmed desorption, and CO temperature-programmed desorption in order to correlate the physicochemical and catalytic properties.

Keywords： Rh2sub>O3sub> CePO4sub> N2sub>O decomposition

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CO2sub> methanation and co-methanation of CO and CO2sub> over Mn-promoted Ni/Al2sub>O3sub> catalysts

Kechao Zhao,Zhenhua Li,Li Bian

Frontiers of Chemical Science and Engineering 2016, Volume 10, Issue 2, Pages 273-280 doi: 10.1007/s11705-016-1563-5

Abstract: A series of Mn-promoted 15 wt-% Ni/Al O catalysts were prepared by an incipient wetness impregnation method. The effect of the Mn content on the activity of the Ni/Al O catalysts for CO methanation and the co-methanation of CO and CO in a fixed-bed reactor was investigated. The catalysts were characterized by N physisorption, hydrogen temperature-programmed reduction and desorption, carbon dioxide temperature-programmed desorption, X-ray diffraction and high-resolution transmission electron microscopy. The presence of Mn increased the number of CO adsorption sites and inhibited Ni particle agglomeration due to improved Ni dispersion and weakened interactions between the nickel species and the support. The Mn-promoted 15 wt-% Ni/Al O catalysts had improved CO methanation activity especially at low temperatures (250 to 400 °C). The Mn content was varied from 0.86% to 2.54% and the best CO conversion was achieved with the 1.71Mn-Ni/Al O catalyst. The co-methanation tests on the 1.71Mn-Ni/Al O catalyst indicated that adding Mn markedly enhanced the CO methanation activity especially at low temperatures but it had little influence on the CO methanation performance. CO methanation was more sensitive to the reaction temperature and the space velocity than the CO methanation in the co-methanation process.

Keywords： Mn promotion nickel catalysts CO2sub> methanation co-methanation of CO and CO2sub>

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A Storage-Driven CO2sub> EOR for a Net-Zero Emission Target Article

Yueliang Liu, Zhenhua Rui

Engineering 2022, Volume 18, Issue 11, Pages 79-87 doi: 10.1016/j.eng.2022.02.010

Abstract: >2sub>) emissions.>2sub> emissions by storing CO2sub> in oil reservoirs.CO2sub> EOR—whose main target is to realize net-zero or even negative CO2sub> emissionsStorage-driven CO2sub> EOR is superior to conventional CO2sub> EOR in improving sweepingthan conventional CO2sub> EOR.

Keywords： CO2sub> EOR Net CO2sub> emissions Dimethyl ether Storage-driven CO2sub> EOR CO2sub> sequestration

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Al2sub>O3sub> and CeO2sub>-promoted MgO sorbents for CO2sub> capture at moderate

Huimei Yu, Xiaoxing Wang, Zhu Shu, Mamoru Fujii, Chunshan Song

Frontiers of Chemical Science and Engineering 2018, Volume 12, Issue 1, Pages 83-93 doi: 10.1007/s11705-017-1691-6

Abstract: A series of Al O and CeO modified MgO sorbents was prepared and studied for CO sorption at moderate temperatures. The CO sorption capacity of MgO was enhanced with the addition of either Al O or CeO . Over Al O -MgO sorbents, the best capacity of 24.6 mg-CO /g-sorbent was attained at 100 °C, which was 61% higher than that of MgO (15.3 mg-CO /g-sorbent). The highest capacity of 35.3 mg-CO /g-sorbent was obtained over the CeO -MgO sorbents at the optimal temperature of 200 °C. Combining with the characterization results, we conclude that the promotion effect on CO sorption with the addition of Al O and CeO can be attributed to the increased surface area with reduced MgO crystallite size. Moreover, the addition of CeO increased the basicity of MgO phase, resulting in more increase in the CO capacity than Al O promoter. Both the Al O -MgO and CeO -MgO sorbents exhibited better cyclic stability than MgO over the course of fifteen CO sorption-desorption cycles. Compared to Al O , CeO is more effective for promoting the CO capacity of MgO. To enhance the CO capacity of MgO sorbent, increasing the basicity is more effective than the increase in the surface area.

Keywords： CO2sub> capture MgO sorbents Al2sub>O3sub> CeO2sub> flue gas

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ZnFe2sub>O4sub> deposited on BiOCl with exposed (001) and (010) facets for photocatalyticreduction of CO2sub> in cyclohexanol

Guixian Song, Xionggang Wu, Feng Xin, Xiaohong Yin

Frontiers of Chemical Science and Engineering 2017, Volume 11, Issue 2, Pages 197-204 doi: 10.1007/s11705-016-1606-y

Abstract: ZnFe O -BiOCl composites were prepared by both hydrothermal and direct precipitation processes and the structures and properties of the samples were characterized by various instrumental techniques. The samples were then used as catalysts for the photocatalytic reduction of CO in cyclohexanol under ultraviolet irradiation to give cyclohexanone (CH) and cyclohexyl formate (CF). The photocatalytic CO reduction activities over the hydrothermally prepared ZnFe O -BiOCl composites were higher than those over the directly-precipitated composites. This is because compared to the direct-precipitation sample, the ZnFe O nanoparticles in the hydrothermal sample were smaller and more uniformly distributed on the surface of BiOCl and so more heterojunctions were formed. Higher CF and CH yields were obtained for the pure BiOCl and BiOCl composite samples with more exposed (001) facets than for the samples with more exposed (010) facets. This is due to the higher density of oxygen atoms in the exposed (001) facets, which creates more oxygen vacancies, and thereby improves the separation efficiency of the electron-hole pairs. More importantly, irradiation of the (001) facets with ultraviolet light produces photo-generated electrons which is helpful for the reduction of CO to ·CO . The mechanism for the photocatalytic reduction of CO in cyclohexanol over ZnFe O -BiOCl composites with exposed (001) facets involves electron transfer and carbon radical formation.

Keywords： reduction of CO2sub> cyclohexanol ZnFe2sub>O4sub> deposited BiOCl facet composite

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The stabilization effect of Al2sub>O3sub> on unconventional Pb/SiO2sub> catalyst

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 10, Pages 1423-1429 doi: 10.1007/s11705-023-2315-y

Abstract: To enhance the stability, the traditional carrier Al2sub>O3sub> with a small amount, wasintroduced into Pb/SiO2sub> catalyst in this study.It has been proved that Al2sub>O3sub> can inhibit the reduction of PbO, and weaken theAs a result, 3Al15Pb/SiO2sub> catalyst exhibits a much higher stability up to more than 150 h.>2sub>O3sub> addition was also proposed.

Keywords： Pb/SiO2sub> Al2sub>O3sub> propane dehydrogenation propene stability

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Cu-doped Bi/Bi2sub>WO6sub> catalysts for efficient N2sub> fixation by photocatalysis

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 10, Pages 1412-1422 doi: 10.1007/s11705-023-2312-1

Abstract: it in photocatalytic N2sub> immobilization.>2sub>WO6sub> composite.>2sub>WO6sub>.>2sub>WO6sub>, respectively.>2sub>-to-NH3sub> conversion.

Keywords： Bi2sub>WO6sub> Cu doping work function photocatalytic N2sub> fixation charge

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Development of H2sub>O/CO2sub> co-electrolysis in solid oxide electrolysis cell

Fan Hui,Song Shidong,Han Minfang

Strategic Study of CAE 2013, Volume 15, Issue 2, Pages 107-112

Abstract: The structure of SOEC, the recent development of high temperature steam/CO2 co-electrolysis from

Keywords： SOEC H2sub>O/CO2sub> co-electrolysis syngas electrolysis efficiency water electrolysis

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Electrochemical oxidation of humic acid at the antimony- and nickel-doped tin oxide electrode

TANG Chengli,YAN Wei,ZHENG Chunli

Frontiers of Environmental Science & Engineering 2014, Volume 8, Issue 3, Pages 337-344 doi: 10.1007/s11783-013-0545-9

Abstract: acid (HA) in aqueous solution by electrochemical oxidation with Antimony- and Nickel-doped Tin oxide electrode(Ni-Sb-SnO /Ti electrode) as the anode.

Keywords： electrochemical oxidation humic acid (HA) natural water Ni-Sb-SnO2sub>/Ti electrode

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Title Author Date Type Operation

Enhancement of the electrocatalytic oxidation of antibiotic wastewater over the conductive black carbon-PbO

Xiangyu Wang, Yu Xie, Guizhen Yang, Jiming Hao, Jun Ma, Ping Ning

Journal Article

NiCo2O4@quinone-rich N–C core–shell nanowires as composite electrode for electric double layer capacitor

Journal Article

Construction of nitrogen-doped carbon cladding LiMnO film electrode with enhanced stability for electrochemically

Journal Article

Construction of NiCoO nanoflake arrays on cellulose-derived carbon nanofibers as a freestanding electrode

Journal Article

A 3D porous WP2 nanosheets@carbon cloth flexible electrode for efficient electrocatalytic hydrogen evolution

Mingyu Pi, Xiaodeng Wang, Dingke Zhang, Shuxia Wang, Shijian Chen

Journal Article

Dielectric barrier micro-plasma reactor with segmented outer electrode for decomposition of pure CO

Baowei Wang, Xiaoxi Wang, Bo Zhang

Journal Article

Rh2sub>O3sub>/hexagonal CePO4sub> nanocatalysts for N2sub>O decomposition

Huan Liu, Zhen Ma

Journal Article

CO2sub> methanation and co-methanation of CO and CO2sub> over Mn-promoted Ni/Al2sub>O3sub> catalysts

Kechao Zhao,Zhenhua Li,Li Bian

Journal Article

A Storage-Driven CO2sub> EOR for a Net-Zero Emission Target

Yueliang Liu, Zhenhua Rui

Journal Article

Al2sub>O3sub> and CeO2sub>-promoted MgO sorbents for CO2sub> capture at moderate

Huimei Yu, Xiaoxing Wang, Zhu Shu, Mamoru Fujii, Chunshan Song

Journal Article

ZnFe2sub>O4sub> deposited on BiOCl with exposed (001) and (010) facets for photocatalyticreduction of CO2sub> in cyclohexanol

Guixian Song, Xionggang Wu, Feng Xin, Xiaohong Yin

Journal Article

The stabilization effect of Al2sub>O3sub> on unconventional Pb/SiO2sub> catalyst

Journal Article

Cu-doped Bi/Bi2sub>WO6sub> catalysts for efficient N2sub> fixation by photocatalysis

Journal Article

Development of H2sub>O/CO2sub> co-electrolysis in solid oxide electrolysis cell

Fan Hui,Song Shidong,Han Minfang

Journal Article

Electrochemical oxidation of humic acid at the antimony- and nickel-doped tin oxide electrode

TANG Chengli,YAN Wei,ZHENG Chunli

Journal Article

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